Moloi is a surname. Notable people with the surname include:
Dirang Moloi (born 1985), Botswanan footballer Lerato Moloi, South African fashion model Mpho Moloi (born 1983), South African footballer Pontsho Moloi (born 1981), Botswanan footballer Precious Moloi-Motsepe, South African fashion entrepreneur and philanthropist Teboho Moloi (born 1968), South African footballer Thabo Moloi (born 1994), South African footballer Timothy Moloi (born 1975), South African singer