Charles Alfred Jeffreys (7 December 1877 – 18 October 1917) was a South African sport shooter who competed in the 1912 Summer Olympics.

In the 1912 Summer Olympics he participated in the following events:

Team military rifle – fourth place 300 metre military rifle, three positions – 34th place 600 metre free rifle – 42nd place 300 metre free rifle, three positions – 70th place

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